Global tropospheric ozone responses to reduced NO(x) emissions linked to the COVID-19 worldwide lockdowns

Miyazaki, Kazuyuki; Bowman, Kevin; Sekiya, Takashi; Takigawa, Masayuki; Neu, Jessica L.; Sudo, Kengo; Osterman, Greg; Eskes, Henk

Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO(x) emissions dropped by at least 15% globally and 18 to 25% regionally in April and May 2020, which decreased free tropospheric ozone by up to 5 parts per billion, consistent with independent satellite observations. The global total tropospheric ozone burden declined by 6TgO(3) (∼2%) in May and June 2020, largely due to emission reductions in Asia and the Americas that were amplified by regionally high ozone production efficiencies (up to 4 TgO(3)/TgN). Our results show that COVID-19 mitigation left a global atmospheric imprint that altered atmospheric oxidative capacity and climate radiative forcing, providing a test of the efficacy of NO(x) emissions controls for co-benefiting air quality and climate.